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Title:
Magnetic properties of actinide elements having the 5f6 and 5f7 electronic configurations
Authors:
Nave, S. E.; Haire, R. G.; Huray, Paul G.
Affiliation:
AA(Physics Department, University of Tennessee, Knoxville, Tennessee 37996), AB(Transuranium Research Laboratory, Chemistry Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830), AC(Physics Department, University of Tennessee, Knoxville, Tennessee 37996)
Publication:
Physical Review B (Condensed Matter), Volume 28, Issue 5, September 1, 1983, pp.2317-2327 (PhRvB Homepage)
Publication Date:
09/1983
Origin:
AIP; APS
DOI:
10.1103/PhysRevB.28.2317
Bibliographic Code:
1983PhRvB..28.2317N

Abstract

Magnetic susceptibility measurements have been made on multimicrogram quantities of 243AmF3, 248CmF4, 248CmO2, and 248CmBaO3 samples (nominally the 5f6 electronic configuration) and on 248Cm2O3, 248CmF3, 249BkF4, and 249BkO2 (nominally the 5f7 electronic configuration) in the temperature range 4.2-300 K and in magnetic fields up to 1650 G. The experimentally determined effective magnetic moments and the Curie-Weiss constants for these compounds are presented. The deviation of the moments for the 5f6 compounds from those expected from classic theory is discussed in terms of low-lying excited states, chemical composition, crystal-field perturbations, and realistic electronic structure.
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